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Exceptionally high turnover frequencies recorded for a new chitosan-based palladium(II) catalyst

Applied Catalysis A: General · Ağustos 2016

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Exceptionally high turnover frequencies recorded for a new chitosan-based palladium(II) catalyst
Applied Catalysis A: General · 2016 SCI
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Makale Bilgileri

DergiApplied Catalysis A: General
Yayın TarihiAğustos 2016
Cilt / Sayfa523 · 12-20
Özet To be industrially feasible, and applicable in synthesis of fine chemicals, a catalyst has to possess high turnover number (TON) and turnover frequency (TOF). In this study, a new cross-linked chitosan derivative was synthesized by using 2,2′-pyridil as a cross-linking agent. 2,2′-Pyridil cross-linked chitosan was used to as a support material for palladium catalyst. Chitosan-pyridil-based Pd(II) catalyst was tested in the microwave-assisted synthesis of biaryls via Suzuki coupling reactions. The catalyst yielded remarkable TONs of up to 20,000 and TOFs of up to 240,964 by using very low catalyst loading (5 × 10-3% mol) in a short reaction time (5 min). The catalyst also showed a better recyclability.

Yazarlar (4)

1
Talat Baran
2
Idris Sargin
ORCID: 0000-0003-3785-9575
3
Ayfer Menteş
4
Murat Kaya

Anahtar Kelimeler

Cross-linking Pyridil Suzuki coupling TOF TON

Kurumlar

Aksaray Üniversitesi
Aksaray Turkey

Metrikler

52
Atıf
4
Yazar
5
Anahtar Kelime

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