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Optical, Optoelectronic, and Third-Order Nonlinear Photonics of Ultrathin Molybdenum Oxide Film Deposited by Atomic Layer Deposition

Physica Status Solidi (A) Applications and Materials Science · Mart 2023

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YÖKSİS Kayıtları
Optical, Optoelectronic, and Third‐Order Nonlinear Photonics of Ultrathin Molybdenum Oxide Film Deposited by Atomic Layer Deposition
PHYSICA STATUS SOLIDI A-APPLICATIONS AND MATERIALS SCIENCE · 2023 SCI-Expanded
DOÇENT YASEMİN GÜNDOĞDU KABAKCI →
Optical, Optoelectronic, and Third‐Order Nonlinear Photonics of Ultrathin Molybdenum oxide Film Deposited by Atomic Layer Deposition
physica status solidi (a) – applications and materials science · 2023 SCI-Expanded
DOÇENT YASEMİN GÜNDOĞDU KABAKCI →

Makale Bilgileri

DergiPhysica Status Solidi (A) Applications and Materials Science
Yayın TarihiMart 2023
Cilt / Sayfa220
Özet The atomic layer deposition (ALD) technique has attracted significant attention because it enables the control of film synthesis at the subnanometre scale. Herein, molybdenum oxide (MoO3) ultrathin films using the ALD system through Bis(t-butylimido)bis(dimethylamino)molybdenum (VI) as a molybdenum (Mo) source are prepared. To understand the effect of deposition temperature, thin films are prepared at three different temperatures 100, 150, and 250 °C. The morphological and elemental properties are assessed using a field emission scanning electron microscope, scanning transmission electron microscopy, and energy-dispersive X-ray spectroscopy techniques. It is observed that the film thicknesses increase with the increase in the deposition temperature. It is found that the film growth at 150 °C is the most potential one for UV optoelectronic applications with high stability even under low applied bias voltages. Moreover, these films show interesting nonlinear optical behaviors as investigated with the z-scan technique applying open and closed aperture methods. The calculated nonlinear optical parameters including nonlinear absorption coefficient (β), nonlinear refractive index (n 2), nonlinear refractive coefficient (γ), and third-order nonlinear susceptibility (χ (3)) are 10−11 m W−1, 10−16 cm2 W−1, 10−11 cm2 W−1, and 10−11 esu, respectively.

Yazarlar (4)

1
Mohamed A. Mohamed
ORCID: 0000-0001-8473-8253
2
Yasemin Gündoğdu
3
Hamdi Şükür Kılıç
4
Yasin Eker

Anahtar Kelimeler

atomic layer deposition MoO 3 nonlinear optics. ultrathin metal oxide thin films z -scan

Kurumlar

Necmettin Erbakan Üniversitesi
Meram Turkey
Selçuk Üniversitesi
Selçuklu Turkey
Solar and Space Research Department
Helwan Egypt

Metrikler

6
Atıf
4
Yazar
5
Anahtar Kelime