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Excited state energies, orbital energies and virial coefficients in Confined multi-electron systems

Journal of Luminescence · Kasım 2022

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Excited state energies, orbital energies and virial coefficients in Confined multi-electron systems
Journal of Luminescence · 2022 SCI
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Makale Bilgileri

DergiJournal of Luminescence
Yayın TarihiKasım 2022
Cilt / Sayfa251
Özet In the present study, the electronic structure of neutral He and Li atoms confined at the center of an impenetrable spherical cavity of varying radius has been investigated. Average, state, orbital energies and wave functions for the ground and excited state electron configurations 1snl (1s2nl)[n = 2, 3, 4 and l = 0, 1, 2 and 3] have been calculated using the method that is a combination of quantum genetic algorithm procedure and Hartree-Fock Roothaan. The atomic orbitals built up from Slater-type orbitals are used in calculations. The average state and orbital energies have been calculated for the first time for the higher excited states with nl [n = 3,4 and l = 1,2,3 for confined He atom and n = 3,4 and l = 0, 1,2,3 for confined Li atom]. The results show that impurity charge and spatial confinement have a great impact on orbital energies, average, state energies and virial coefficients of the system, especially in strong confinement region. In addition, it is seen that when cavity radius is extremely large, all state energies and virial coefficients approach the corresponding values of free atom.

Yazarlar (4)

1
Celalettin Demir
2
Yusuf Yakar
3
Bekir Çakir
4
Ayhan Özmen

Anahtar Kelimeler

Average state energy Confined many-electron systems Orbital energy Virial coefficient

Kurumlar

Aksaray Üniversitesi
Aksaray Turkey
Selçuk Üniversitesi
Selçuklu Turkey

Metrikler

5
Atıf
4
Yazar
4
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